欢迎登录材料期刊网

材料期刊网

高级检索

Fe-g-C3N4-LUS-1was prepared by the thermal decomposition of dicyandiamide inside the pores of LUS-1under an inert atmosphere.It was used as a photocatalyst for the hydroxylation of benzene to phenol in sunlight.The catalysts were characterized by Fourier transform infrared spectroscopy,N2 adsorption-desorption,X-ray diffraction,and scanning electron microscopy.In Fe-g-C3N4-LUS-1,a single layer of graphitic carbon nitride (g-C3N4) was formed on the surface of LUS-1.The photocatalytic activity of the iron containing g-C3N4based catalysts was investigated,and the catalytic activity was remarkably enhanced when the reaction condition was changed from dark to sunlight.The best result was obtained with 20%Fe-g-C3N4-LUS-1 in sunlight.

参考文献

[1] Pan J H;Dou H;Xiong Z;Xu C Ma J Zhao X S .[J].Journal of Materials Chemistry,2010,20:451.
[2] Wang J;Li RH;Zhang ZH;Sun W;Xu R;Xie YP;Xing ZQ;Zhang XD .Efficient photocatalytic degradation of organic dyes over titanium dioxide coating upconversion luminescence agent under visible and sunlight irradiation[J].Applied Catalysis, A. General: An International Journal Devoted to Catalytic Science and Its Applications,2008(1/2):227-233.
[3] Goettmann F;Fischer A;Antonietti M;Thomas A .[J].New Journal of Chemistry,2007,31:1455.
[4] Pan H;Li X;Zhuang Z;Zhang C .[J].JMol CatalA,2011,345:90.
[5] Sun J H;Dong S Y;Feng J L;Yin X J Zhao X C .[J].Journal of Molecular Catalysis A:Chemical,2011,335:145.
[6] Li K;Martin D;Tang J .[J].Chinese Journal of Catalysis,2011,32:879.
[7] Oh W-C;Chen M;Cho K;Kim C Meng Z Zhu L .[J].Chinese Journal of Catalysis,2011,32:1577.
[8] Xiao Y;Dang L;An L;Bai S Lei Z .[J].Chinese Journal of Catalysis,2008,29:31.
[9] Ao Y;Xu J;Zhang S;Fu D .[J].Journal of Physics and Chemistry of Solids,2009,70:1042.
[10] Guan G;Kida T;Yoshida A .[J].Applied Catalysis B:Environmental,2003,41:387.
[11] Kuai, L.;Geng, B.;Chen, X.;Zhao, Y.;Luo, Y. .Facile subsequently light-induced route to highly efficient and stable sunlight-driven Ag-AgBr plasmonic photocatalyst[J].Langmuir: The ACS Journal of Surfaces and Colloids,2010(24):18723-18727.
[12] Vidya K;Kamble VS;Selvam P;Gupta NM .Uranyl-anchored MCM-41 as a highly efficient photocatalyst for the complete oxidation of methanol under sunlight[J].Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications,2004(3):145-154.
[13] Hou LR;Yuan CZ;Peng Y .Preparation and photocatalytic property of sunlight-driven photocatalyst Bi38ZnO58[J].Journal of molecular catalysis, A. Chemical,2006(1/2):132-135.
[14] Nezamzadeh-Ejhieh A;Hushmandrad S .[J].Applied Catalysis A:General,2010,388:149.
[15] Sonawane RS;Dongare MK .Sol-gel synthesis of Au/TiO2 thin films for photocatalytic degradation of phenol in sunlight[J].Journal of molecular catalysis, A. Chemical,2006(1):68-76.
[16] Wang Z-Y;Chou H-C;Wu J C S;Tsai D P Mul G .[J].Applied Catalysis A:General,2010,380:172.
[17] Ke D;Peng T;Ma L;Cai P Jiang P .[J].Applied Catalysis A:General,2008,350:111.
[18] Chen X;Zhang J;Fu X;Antonietti M Wang X .[J].Journal of the American Chemical Society,2009,131:11658.
[19] Zhang J;Chen X;Takanabe K;Maeda K,Domen K,Epping J D,Fu X,Antonieta M,Wang X .[J].Angewandte Chemie International Edition,2010,49:441.
[20] Thomas A;Fischer A;Goettmann F;Antonietti M Müller J O Schl(f)gl R Carlsson J M .[J].Journal of Materials Chemistry,2008,18:4893.
[21] Komatsu T. .Attempted chemical synthesis of graphite-like carbon nitride[J].Journal of Materials Chemistry: An Interdisciplinary Journal dealing with Synthesis, Structures, Properties and Applications of Materials, Particulary Those Associated with Advanced Technology,2001(3):799-801.
[22] Komatsu T. .The first synthesis and characterization of cyameluric high polymers[J].Macromolecular chemistry and physics,2001(1):19-25.
[23] Zhang Z;Leinenweber K;Bauer M;Garvie L A J McMillan P F WolfG H .[J].Journal of the American Chemical Society,2001,123:7788.
[24] Guo Q;Xie Y;Wang X;Lv S Hou T Liu X .[J].Chemical Physics Letters,2003,380:84.
[25] Montigaud H.;Demazeau G.;Alves I.;Courjault S.;Tanguy B. .C3N4: Dream or reality ?<Tau Beta > Solvothermal synthesis as macroscopic samples of the C3N4 graphitic form[J].Journal of Materials Science,2000(10):2547-2552.
[26] Lotsch B V;Schnick W .[J].Chemistry of Materials,2006,18:1891.
[27] Bojdys MJ;Muller JO;Antonietti M;Thomas A .Ionothermal Synthesis of Crystalline, Condensed, Graphitic Carbon Nitride[J].Chemistry: A European journal,2008(27):8177-8182.
[28] Montigaud H;Tanguy B;Demazeau G;Alves I Birot M Dunogues J .[J].Diamond and Related Materials,1999,8:1707.
[29] Bai Y J;Lü B;Liu Z G;Li L Cui D L Xu X G Wang Q L .[J].Journal of Crystal Growth,2003,247:505.
[30] Zhao H;Chen X L;Jia C;Zhou T Qu X Jian J Xu Y .[J].Materials Science and Engineering B,2005,122:226.
[31] Li X;Zhang J;Shen L;Ma Y Lei W Cui Q Zou G .[J].Applied Physics A:Materials Science and Processing,2009,94:387.
[32] Yan, SC;Li, ZS;Zou, ZG .Photodegradation of Rhodamine B and Methyl Orange over Boron-Doped g-C3N4 under Visible Light Irradiation[J].Langmuir: The ACS Journal of Surfaces and Colloids,2010(6):3894-3901.
[33] Yan, S. C.;Li, Z. S.;Zou, Z. G. .Photodegradation Performance of g-C3N4 Fabricated by Directly Heating Melamine[J].Langmuir,2009(17):10397-10401.
[34] Gholami J;Badiei A;Abbasi A;Ziarani G M .[J].Int J Chem Tech Res,2009,1:426.
[35] Martínez F;Calleja G;Melero J A;Molina R .[J].Applied Catalysis B:Environmental,2005,60:181.
[36] Sirotin S V;Moskovskaya I F .[J].Petroleum Chemistry,2009,49:99.
[37] Badiei A;Bonneviot L;Crowther N;Ziarani GM .Surface tailoring control in micelle templated silica[J].Journal of Organometallic Chemistry,2006(26):5911-5919.
[38] Arab P;Badiei A;Koolivand A;Mohammadi Ziarani G .[J].Chinese Journal of Catalysis,2011,32:258.
[39] Franklin E C .[J].Journal of the American Chemical Society,1922,44:486.
[40] Wang X;Chen X;Thomas A;Fu X Antonietti M .[J].Advanced Materials,2009,21:1609.
[41] Guo Q;Xie Y;Wang X;Zhang S,Hou T,Lv S.[J].Chemical Communications,2004:26.
上一张 下一张
上一张 下一张
计量
  • 下载量()
  • 访问量()
文章评分
  • 您的评分:
  • 1
    0%
  • 2
    0%
  • 3
    0%
  • 4
    0%
  • 5
    0%