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催化学报 , 2012, 33(1): 51-59. doi: 10.3724/SP.J.1088.2012.10764

含氮分子筛的研究进展

武光军 1, , 关乃佳 2, , 李兰冬 3,

1.南开大学化学学院先进能源材料化学教育部重点实验室,天津300071

2.南开大学化学学院先进能源材料化学教育部重点实验室,天津300071

3.南开大学化学学院先进能源材料化学教育部重点实验室,天津300071

基金项目:   国家重点基础研究发展计划(973计划)(2009CB623502)  

关键词： 含氮分子筛 , 表面酸碱性 , 氮含量 , 氮化机理 , 催化性能 , 理论计算

Recent Development of Nitrogen-Incorporated Molecular Sieves

含氮分子筛作为一种新型的含骨架杂原子分子筛,具有择形碱催化作用和酸碱双功能催化作用,近年来引起了人们广泛的研究兴趣.本文总结了微孔和介孔含氮分子筛在制备、表征和催化性能等方面的研究现状,重点评述了氮化机理和理论计算在含氮分子筛研究中的应用,并展望了含氮分子筛今后的研究方向.

参考文献

[1] 徐如人;庞文琴;于吉红;霍启升,陈接胜.分子筛与多孔材料化学[M].北京:科学出版社,2004
[2] Hattori H .[J].Chemical Reviews,1995,95:537.
[3] 宋艳,李永红.介孔分子筛的应用研究新进展[J].化学进展,2007(05):659-664.
[4] 胥月兵,陆江银,钟梅,王吉德.ZSM-5分子筛在低碳烷烃脱氢中的催化应用[J].化学进展,2008(05):650-656.
[5] 岳明波,朱建华.从介孔分子筛原粉研制高效吸附二氧化碳的有机胺-介孔复合材料[J].催化学报,2008(10):1051-1057.
[6] 谢伟,刘月明,汪玲玲,吴鹏.具有MWW结构钛硅分子筛的研究进展[J].催化学报,2010(05):502-513.
[7] Yao S;Sun C;Li J;Huang X Shen W .[J].Journal of Natural Gas Chemistry,2010,19:1.
[8] Sun D;Li X;Ji S;Cao L .[J].Journal of Natural Gas Chemistry,2010,19:369.
[9] Agarwal, V.;Huber, G.W.;Conner Jr., W.C.;Auerbach, S.M. .DFT study of nitrided zeolites: Mechanism of nitrogen substitution in HY and silicalite[J].Journal of Catalysis,2010(1):53-63.
[10] Yamamoto K;Tatsumi T .[J].Chemistry of Materials,2008,20:972.
[11] Kerr T G;Shipman R G .[J].Journal of Physical Chemistry,1968,72:3071.
[12] Hammond KD;Dogan F;Tompsett GA;Agarwal V;Conner WC;Grey CP;Auerbach SM .Spectroscopic Signatures of Nitrogen-Substituted Zeolites[J].Journal of the American Chemical Society,2008(45):14912-14913.
[13] Dogan, F;Hammond, KD;Tompsett, GA;Huo, H;Conner, WC;Auerbach, SM;Grey, CP .Searching for Microporous, Strongly Basic Catalysts: Experimental and Calculated Si-29 NMR Spectra of Heavily Nitrogen-Doped Y Zeolites[J].Journal of the American Chemical Society,2009(31):11062-11079.
[14] Srasra M;Delsarte S;Gaigneaux E M .[J].Topics in Catalysis,2009,52:1541.
[15] Hammond K D;Gharibeh M;Tompsett G A;Dogan F Brown A V Grey C P Auerbach S M Conner W C Jr .[J].Chemistry of Materials,2010,22:130.
[16] Srasra M;Delsarte S;Gaigneaux E M .[J].Journal of Physical Chemistry C,2010,114:4527.
[17] Wang T;Li L;Wu G;Guan N .[J].Advances in Materials Research,2011,148-149:957.
[18] 王涛,武光军,李兰冬,关乃佳.含氮FAU分子筛的制备、表征及碱催化反应性能[J].高等学校化学学报,2011(03):743-747.
[19] Shen W;Tompsett G A;Hammond K D;Xing R'Dogan F Grey C P Conner W C Jr Auerbach S M Huber G W .[J].Applied Catalysis A:General,2011,392:57.
[20] Ernst S.;Sauerbeck S.;Bongers T.;Hartmann M. .A novel family of solid basic catalysts obtained by nitridation of crystalline microporous aluminosilicates and aluminophosphates[J].Applied Catalysis, A. General: An International Journal Devoted to Catalytic Science and Its Applications,2000(1/2):117-123.
[21] Zhang C;Xu Z;Wan K;Liu Q .[J].Applied Catalysis A:General,2004,258:55.
[22] Guan X X;Li N;Wu G J;Chen J X Zhang F X Guan N J .[J].Journal of Molecular Catalysis A:Chemical,2006,248:220.
[23] 关新新,李娜,武光军,章福祥,陈继新,关乃佳.HZSM-5的氮化及其在乙苯与乙醇烷基化反应中的应用[J].催化学报,2005(08):634-636.
[24] Hasegawa T;Krishnan C K;Ogura M .[J].Microporous and Mesoporous Materials,2010,132:290.
[25] Wu G J;Wang X;Yang Y L;Li L D Wang G Guan N J .[J].Microporous and Mesoporous Materials,2010,127:25.
[26] 丁云杰;熊建民;吕元;何新生 林励吾 .[J].催化学报,2001,22:227.
[27] Narasimharao, K;Hartmann, M;Thiel, HH;Ernst, S .Novel solid basic catalysts by nitridation of zeolite beta at low temperature[J].Microporous and Mesoporous Materials,2006(1/3):377-383.
[28] Xiong J M;Ding Y J;Zhu H;Yah L Liu X Lin L W .[J].Journal of Physical Chemistry B,2003,107:1366.
[29] Guan X X;Zhang F X;Wu G J;Guan N J .[J].Materials Letters,2006,60:3141.
[30] 关新新,武光军,刘克成,章福祥,关乃佳.含N微孔SAPO-34分子筛的制备、表征及催化性能[J].石油学报(石油加工),2007(01):15-19.
[31] Regli L;Bordiga S;Busco C;Prestipino C Ugliengo P Zecchina A Lamberti C .[J].Journal of the American Chemical Society,2007,129:12131.
[32] Li H;Lei Q;Zhang X;Suo J .[J].Chem Cat Chem,2010,3:145.
[33] Inaki Y;Kajita Y;Yoshida H;Ito K,Hattori T.[J].Chemical Communications,2001:2358.
[34] El Haskouri J;Cabrera S;Sapi(n)a F;Latorre J Guillem C Beltrán-Porter A Beltrán-Porter D Marcos D Amorós P .[J].Advanced Materials,2001,13:192.
[35] Xia Y;Mokaya R .[J].Journal of Materials Chemistry,2004,14:2507.
[36] Zhang CM;Liu Q;Xu Z .Synthesis and characterization of non-crystalline mesoporous silicon oxynitride MCM-41 with high nitrogen content[J].Journal of Non-Crystalline Solids: A Journal Devoted to Oxide, Halide, Chalcogenide and Metallic Glasses, Amorphous Semiconductors, Non-Crystalline Films, Glass-Ceramics and Glassy Composites,2005(16/17):1377-1382.
[37] 张存满,刘茜,徐政.具有碱催化活性的有序氮氧化硅MCM-41介孔分子筛的制备与性能研究[J].化学学报,2006(04):313-319.
[38] 蒋绍亮,宋英俊,章福祥,武光军,关乃佳.高氮含量MCM-41的制备及其对Knoevenagal缩合反应的催化性能[J].催化学报,2006(06):495-500.
[39] Ishizu K;Hayashi F;Iwamoto M .[J].Chemistry Letters,2007,36:1416.
[40] Hayashi F;Ishizu K;Iwamoto M .[J].Journal of the American Ceramic Society,2010,93:104.
[41] Wu G J;Jiang Sh L;Li L D;Zhang F X Yang Y L Guan N J Mihaylov M Kn(o)zinger H .[J].Microporous and Mesoporous Materials,2010,135:2.
[42] Hayashi, F.;Ishizu, K.-I.;Iwamoto, M. .Effect of pore structure on the nitridation of mesoporous silica with ammonia[J].European journal of inorganic chemistry,2010(15):2235-2243.
[43] Xia Y;Mokaya R .[J].Angewandte Chemie International Edition,2003,42:2639.
[44] Xia Y;Mokaya R .[J].JPhys Chem C,2008,112:1455.
[45] Wan K;Liu Q;Zhang C .[J].Chemistry Letters,2003,32:362.
[46] Wan K;Liu Q;Zhang C;Wang J .[J].Bulletin of the Chemical Society of Japan,2004,77:1409.
[47] Wang J;Liu Q .[J].Microporous and Mesoporous Materials,2005,83:225.
[48] Chino N;Okubo T .[J].Microporous and Mesoporous Materials,2005,87:15.
[49] Wang M;Liu Q;Wang J;Xiu T .[J].Journal of the American Ceramic Society,2008,91:2405.
[50] Zhao Y;Qi Y;Zhang Y;Zhang S Liu Z .[J].Materials Letters,2008,62:1197.
[51] Zhao Y;Qi Y;Wei Y;Zhang Y Zhang S Yang Y Liu Z .[J].Microporous and Mesoporous Materials,2008,111:300.
[52] Wu G J;Jiang Sh L;Li L D;Guan N J .[J].Applied Catalysis A:General,2011,391:225.
[53] Wang T;Wu G J;Guan N J;Li L D .[J].Microporous and Mesoporous Materials,2012,148:184.
[54] 关乃佳;李牛;武光军;杨雅莉.新结构高性能多孔催化材料[M].北京:中国石化出版社,2010:28.
[55] Paparatto G;Moretti E;Leofanti G;Gatti F .[J].Journal of Catalysis,1987,105:227.
[56] Kim J H;Namba S;Yashima T .[J].Bulletin of the Chemical Society of Japan,1988,61:1051.
[57] Wang I;Ay C L;Lee B J;Chen M H .[J].Applied Catalysis,1989,54:257.
[58] Kim J H;Namba S;Yashima T .[J].Applied Catalysis A:General,1992,83:51.
[59] Miyamoto A;Kobayashi Y;Elanany M;Tsuboi H Koyama M Endou A Takaba H Kubo M Carpio C A D Selvam P .[J].Microporous and Mesoporous Materials,2007,101:324.
[60] Smit B;Maesen T L M .[J].Chemical Reviews,2008,108:4125.
[61] Corma A.;Fernandez L.;Pedro V. .Structural incorporation of nitrogen into zeolites, and alpos: Ab initio molecular orbital calculations on stability and basicity[J].Journal of molecular catalysis, A. Chemical,1998(3):241-250.
[62] Astala R;Auerbach S M .[J].Journal of the American Chemical Society,2004,126:1843.
[63] Elanany M;Su BL;Vercauteren DP .The effect of framework organic moieties on the acidity of zeolites: A DFT study[J].Journal of molecular catalysis, A. Chemical,2007(1/2):195-199.
[64] Agarwal V;Conner W C Jr;Auerbach S M .[J].Journal of Physical Chemistry C,2011,115:188.
[65] Lesthaeghe D;Van Speybroeck V;Waroquier M .[J].Journal of the American Chemical Society,2004,126:9162.
[66] Lesthaeghe D;Van Speybroeck V;Marin B G;Waroquier M .[J].Journal of Physical Chemistry B,2005,109:7952.
[67] Zheng A;Wang L;Chen L;Yue Y Ye C Lu X Deng F .[J].ChemPhysChem:A European Journal of Chemical Physics and Physical Chemistry,2007,8:231.
[68] Agarwal, V.;Huber, G.W.;Curtis Conner Jr., W.;Auerbach, S.M. .Kinetic stability of nitrogen-substituted sites in HY and silicalite from first principles[J].Journal of Catalysis,2010(2):249-255.
[69] 武光军,杨雅莉,王贵昌,章福祥,关乃佳.ZSM-5分子筛氮化的密度泛函理论研究[J].催化学报,2008(03):203-205.
[70] 武光军;王鑫;于爱敏;王贵昌 杨雅莉 章福祥 关乃佳 .[J].高等学校化学学报,2009,29:2403.
[71] Chan, B;Radom, L .Zeolite-catalyzed hydrogenation of carbon dioxide and ethene[J].Journal of the American Chemical Society,2008(30):9790-9799.
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