欢迎登录材料期刊网

材料期刊网

高级检索

以粉煤灰和蔗糖为原料,浓硫酸为炭化剂,制备了一种新型的C/粉煤灰复合吸附材料.采用X光电子能谱、红外吸收光谱、场发射扫描电子显微镜、X射线衍射及N2气吸附实验对所制备复合材料进行了表征.结果表明,粉煤灰表面被类石墨态炭纳米颗粒所包裹,复合材料表面密集分布着大量的介孔,Brunauer-Emmett-Teller(BET)比表面积SBET =5.4 m2/g,并且在该复合材料表面含有丰富的-SO3H、-COOH和-OH等含氧官能团.考察了所制备的复合材料对典型阳离子型染料亚甲基蓝及重金属离子的吸附能力,结果表明,该复合材料具有优异的吸附性能,其对亚甲基蓝的吸附能力达到活性炭的83.7%,对典型重金属离子的吸附能力优于市售活性炭.所制备复合材料可作为活性炭的一种替代品,用于水中有机染料和重金属离子的吸附处理.

参考文献

[1] YAO Le.Study on Treatment of Castewater Containing Oil with Fly Ash Modified by PDMDAAC[J].Chinese J Sci Technol Eng,2009,22 (9):6926-6928 (in Chinese).姚乐.PDMDAAC改性粉煤灰吸附处理含油废水实验研究[J].科学技术与工程,2009,22(9):6926-6928.
[2] FU Mingxing,TAN Hongbin,GUO Congsheng,et al.Study on Synthesized Process and Adsorptive Ability of Zeolite P by Coal Fly Ash[J].Bull Chinese Ceram Soc,2009,28(3):468-472(in Chinese).傅明星,谭宏斌,郭从盛,等.粉煤灰制备P型沸石及吸附性能研究[J].硅酸盐通报,2009,28(3):468-472.
[3] HU Zhuannian,YANG Zhiyuan.Cr6 + Adsorption Mechanism on ULTrafine Coal Fly Ashes and Its Kinetics[J].J China Univ Min Technol,2008,37 (4):478-482(in Chinese).刘转年,杨志远.超细粉煤灰吸附Cr6+机理和动力学[J].中国矿业大学学报,2008,37(4):478-482.
[4] Ahnaruzzanan M.A Review on the Utilization of Fly Ash[J].Prog Energy Combust Sci,2010,36(2):327-363.
[5] Wang S,Ma Q,Zhu Z H.Characteristics of Coal Fly Ash and Adsorption Application[J].Fuel,2008,87(15/16):3469-3473.
[6] LIU Zhuannian,WANG Nianqin.Study on the Adsorption Mechanism of Ulrea-fine Coal Fly Ash towards Methylene Blue[J].Chinese J Ion Exch Adsorpt,2008,24(6):535-543(in Chinese).刘转年,王念秦.超细粉煤灰吸附亚甲基蓝的机理研究[J].离子交换与吸附,2008,24(6):535-543.
[7] ZHOU Limin,JIN Jieyun,WANG Yiping,et al.Adsorption of Cd2+ and Ni2+ Ions in Coal Fly Ash[J].Chinese J Fuel Chem Technol,2008,36(5):557-562(in Chinese).周利民,金解云,王一平,等.Cd2+和Ni2+在粉煤灰上的吸附特性[J].燃料化学学报,2008,36(5):557-562.
[8] XI Yonghui.Experimental Study on Sorption of Pb(Ⅱ) with Different Absorbent Materials[J].Chinese J Tongji Univ(Nat Sci),2006,34(9):1226-1230(in Chinese).席永慧.铅离子吸附材料试验研究[J].同济大学学报(自然科学版),2006,34 (9):1226-1230.
[9] Panday K K,Prasad G,Singh V N.Copper(Ⅱ) Removal from Aqueous Solutions by Fly Ash[J].Water Res,1985,19(8):69-73.
[10] Querol X,Moreno N,Uma(n)a J C,et al.Synthesis of Zeolites from Coal Fly Ash:an Overview[J].Int J Coal Geol,2002,5O(1/4):413-423.
[11] Erol M,Kü(c)ükbayrak S,Ersoy-mericboyu A.Comparison of the Properties of Glass,Glass Ceramic and Ceramic Materials Produced from Coal Fly Ash[J].J Hazard Mater,2008,153(1/2):418-425.
[12] Misran H,Singh R,Begum S,et al.Processing of Mesoporous Silica Materials(MCM-41) from Coal Fly Ash[J].J Mater Process Technol,2007,186(1/3):8-13.
[13] XU Jieming,XIE Jimin,ZHU Jianjun.Study on Preparing Nanosized SiO2 ·xH2O from Fly Ash by Gas-phase Method[J].Chinese J lnorg Chem Ind,2006,38(7):54-56(in Chinese).徐洁明,谢吉民,朱建军.粉煤灰气相法制备纳米白炭黑研究[J].无机盐工业,2006,38(7):54-56.
[14] FANG Rongli,WANG Lin.Preparation of High Purity and Ultrafine Aluminum Hydroxide by Using Fly-ash in Ecology[J].Chinese J Chem Eng,2005,33(3):29-32(in Chinese).方荣利,王琳.生态化利用粉煤灰制备高纯超细氢氧化铝[J].化学工程,2005,33 (3):29-32.
[15] Parkh C,Park Y J,Stervens R.Synthesis of Alumina from High Purity Alum Derived from Coal Fly Ash[J].Mater Sci Eng A,2004,367(1):166-170.
[16] Pengthamkeorati P,Satapanajaru T,Chularuengoaksom P.Chemical Modification of Coal Fly Ash for the Removal of Phosphate from Aqueous Solution[J].Fuel,2008,87(12):2469-2476.
[17] Chen C,Zhang P,Zeng G,et al.Sewage Sludge Conditioning with Coal Fly Ash Modified by Sulfuric Acid[J].Chem Eng J,2010,158(3):616-622.
[18] CHEN Guangchun,XI Weiwei,GONG Shuxin,et al.Adsorption of Acid Light Yellow by HDTMA Modified Fly ASh[J].Chinese J Environ Eng,2008,2 (12):1663-1666 (in Chinese).陈广春,席薇薇,龚曙新,等.HDTMA改性粉煤灰吸附酸性嫩黄染料废水[J].环境工程学报,2008,2 (12):1663-1666.
[19] Toda M,Takngaki A,Okamura M,et al.Biodiesel Made with Sugar Catalyst[J].Nature,2005,438(10):178-178.
[20] Zhang D,Luo H,Wang Y,et al.Preparation of Nonporous Carbon-besed Sorbent from Sucrose[J].Chem Lett,2010,39(4):424-425.
[21] Liang X,Zeng M,Qi C.One-step Synthesis of Carbon Functionalized with Sulfonic Acid Groups Using Hydrothermal Carbonization[J].Carbon,2010,48(6):1844-1848.
[22] Suganuma S,Nakajima K,Kitano M,et al.Hydrolysis of Cellulose by Amorphous Carion Bearing SO3H,COOH,and OH Groups[J].J Am Chem Soc,2008,130(38):12787-12793.
[23] Hong R Y,Fu H P,Di G Q,et al.Facile Route to γ-Fe2O3/SiO2 Nanocomposite Used as a Precursor of Magnetic Fluid[J].Mater Chem Phys,2008,108(1):132-141.
[24] Yue Z,Jiang W,Wang L,et al.Surface Characterization of Electrochemically Oxidized Carbon Fibers[J].Carbon,1999,37(11):1785-1796.
[25] Sing g S W,Everett D H,Haul R A W,et al.Reporting Physisorption Data for Gas/Solid Systems with Special Reference to the Determination of Surface Area and Porosity[J].Pure Appl Chem,1985,57(2):603-619.
[26] QIU Mande,YAO Zihua,ZHAI Yongqing,et al.Microanalysis of Fly Ash by SEM and EDS[J].Chinese J Electron Microsc Soc,2008,27(2):112-116(in Chinese).仇满德,姚子华,翟永清,等.粉煤灰的SEM及X射线能谱微分析研究[J].电子显微学报,2008,27(2):112-116.
[27] HUANG Renhe,WANG Li.Study on XRD Spectra of Graphite and Ggraphite/Bismaleimide Antifriction Composites[J].Chinese J Chem Res,2005,16(1):39-58(in Chinese).黄仁和,王力.石墨及石墨/双马来酰亚胺减摩树脂复合材料的XRD研究[J].化学研究,2005,16(1):39-58.
上一张 下一张
上一张 下一张
计量
  • 下载量()
  • 访问量()
文章评分
  • 您的评分:
  • 1
    0%
  • 2
    0%
  • 3
    0%
  • 4
    0%
  • 5
    0%