采用常规的固相反应方法制备了Sr14-xCaxCu24O41系列样品(x=0.0,3.5,6.0,8.4).X-ray衍射结果显示,所有样品均为单相,并且随着掺杂离子含量的增加,样品的晶格常数a,b,c的值均逐渐减小.在10 K～200 K温度范围内测量了不同磁场强度(H=1 T,3 T,5 T)Ca掺杂样品(x=0,3.5,6,8.4)的磁化率温度曲线.磁化率测量结果表明,磁场的增强导致居里-外斯贡献降低,并且导致自旋能隙变小.进一步拟合结果表明,参与磁化率贡献的自旋数目随Ca掺杂浓度的变化不明显,而随磁场强度的增大而减小.
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