介绍了一种高效下转换效应--"量子切割"."量子切割"是由于稀土离子之间的能量传递,使发光材料吸收一个真空紫外光子而放出两个可见光子的过程,为制备高效发光材料提供了新的思路.以Gd3+-Eu3+,Er3+-Gd3+-Tb3+体系为例讨论了"量子切割"机理在发光材料研究方面的一些应用,对其优缺点进行了讨论.
参考文献
[1] | Blasse G, Gramber B C. Luminscent Materials[M].Berlin: Springer-verlag Press, 1994. |
[2] | Henderson B, Imbusch G F. Spectroscopy on Inorganic Solids[M]. Clarendon.Oxford Press, 1989. |
[3] | Ronda C R. Phosphors for lamps and displays: an applicational view [J]. J. Alloys Compd., 1995, 225: 534-538. |
[4] | Rao R P, Devine D J. RE-activated lanthanide phosphate phosphors for PDP applications[J]. J. Lumin., 1999, 87:1260-1263. |
[5] | Kim C H, Kwon Il-Eok, Park C H, et al. Phosphors for plasma display panels[J]. J. Alloys Compd., 2000, 311:33-39. |
[6] | Sommerdijk J L, Bril A, de Jager A W. Luminescence of Pr3+ activated fluorides[J]. J. Lumin., 1974, 9(4):288-296. |
[7] | Piper W W, DeLuca J A, Ham F S. Cascade fluorescent decay in Pr3+ doped fluorides: achievement of a quantum yield greater than unity for emission of visible light[J]. J. Lumin., 1974, 8 (4): 344-348. |
[8] | Doughty D A, Beers W W. Photon cascade luminescence of Pr3+ in LaMgB5O10[J]. J. Electrochem. Soc., 1996, 143:4113-4116. |
[9] | Bhola V P. 4f-5d transition of Pr3+ in CaF2[J]. J. Lumin., 1976, 14(2):115-120. |
[10] | Wegh R T, Donker H, Meijerink A. Vacuum-ultraviolet spectroscopy and quantum cutting for Gd3+ in LiYF4[J]. Physica. Rev. B, 1997, 56(21):13841-13848. |
[11] | Wegh R T, Donker H, Oskam H D, et al. Visible quantum cutting in LiGdF4∶Eu3+ through downconversion[J]. Science, 1999, 283:663-665. |
[12] | Wegh R T, Donker H, van Loef E V D, et al. Quantum cutting through downconversion in rare-earth compounds [J]. J. Lumin., 2000, 87-89:1017-1019. |
[13] | van Vliet J P M, van der Voort D, Blasse G. Luminescence and energy migration in Eu3+-containing scheelites with different anions[J]. J. Lumin., 1989, 42:305-316. |
[14] | Smit W M A, Blasse G. Luminescence and energy migration in the garent Gd3Li3Te2O12 doped with several rare earths and uranium[J]. J. Solid State Chem.,1986, 63(2):308-315. |
[15] | Blasse G, Kiliaan H S, de Vries A J. Study of the energy transfer process in sensitized gadolinium phosphors[J]. J. Less-Common Met., 1986,126:139-146. |
[16] | de Vries A J, Minks B P, Blasse G. Evaluation of the energy migration in GdAl3B4O12[J]. J. Lumin., 1988, 39(3):153-160. |
[17] | Wegh R T, Donker H, Oskam K D, et al. Visible quantum cutting in Eu3+-doped gadolinium fluorides via downconversion[J]. J. Lumin., 1999, 82:93-104. |
[18] | Feldmann C, Jüstel T, Ronda C R, et al. Quantum efficiency of down-conversion phosphor LiGdF4:Eu[J]. J. Lumin., 2001, 92:245-254. |
[19] | Oskam K D, Wegh R T, Donker H, et al. Downconversion: a new route to visible quantum cutting[J]. J. Alloys Comp., 2000, 300-301:421-425. |
[20] | Donker H, Wegh R T, Meijerink A, et al. New concepts for VUV phosphors with high quantum efficiency (q>100%)[J]. J. SID, 1998, 6/1:73-76. |
[21] | Wegh R T, van Loef E V D,Meijerink A.Visible quantum cutting via downconversion in LiGdF4∶Er3+,Tb3+ upon Er3+ 4f11→4f105d excitation [J]. J. Lumin., 2000, 90:111-122. |
[22] | 张俊英.PDP用荧光粉的合成及其发光性能研究[A]. 清华大学博士论文[D].2002. |
[23] | 张庆礼,郭常新,施朝淑.GdVO4∶Eu的激发光谱特性研究[J]. 发光学报,2000,21(4):352-358. |
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