笼型倍半硅氧烷基聚合物是一种典型的多面体有机/无机分子复合物材料,因其具有优异的光、电、热、磁、声、力学和化学相容性等性能,所以近年来被引入较为尖端的技术领域进行研究和应用.本文归纳总结了笼型倍半硅氧烷基聚合物的现行制备方法,讨论了笼型倍半硅氧烷结构对材料性能的影响.最后,对笼型倍半硅氧烷基聚合物材料的应用领域和发展趋势进行了说明.
参考文献
| [1] | Kim KM.;Adachi K.;Chujo Y. .Polymer hybrids of functionalized silsesquioxanes and organic polymers utilizing the sol-gel reaction of tetramethoxysilane[J].Polymer: The International Journal for the Science and Technology of Polymers,2002(4):1171-1175. |
| [2] | Frank J. Feher;Daravong Soulivong;Gregory T. Lewis .Facile Framework Cleavage Reactions of a Completely Condensed Silsesquioxane Framework[J].Journal of the American Chemical Society,1997(46):11323-11324. |
| [3] | Koo J H;Stretz H;Weispfenning A B.44th AIAA/ASME/ASCE/AHS,structures Structural dynamics,and materials conference 7-10 April 2003,Norfolk,Virginia[J].American Institute of Aeronautics and Astronautics,{?}:2003-1769. |
| [4] | Zhang Chunxin .Hydrosilylation of Allyl Alcohol with [HSiMe_2OSiO_(1.5)]_8: Octa(3-hydroxypropyldimethylsiloxy)octasilsesquioxane and Its Octamethacrylate Derivative as Potential Precursors to Hybrid Nanocomposites[J].Journal of the American Chemical Society,2000(29):6979-6988. |
| [5] | J F Brown;L H Vogt;P I Prescott.Preparation and Characterization of the Lower Equilibrated Phenylsilsesquioxanes[J].Journal of the American Chemical Society,1964(86):1120-1125. |
| [6] | A Sellinger;Richard M Laine.Silsesquioxanes as Synthetic Platforms.Thermally Curable and Photocurable Inorganic/Organic Hybrids[J].Macromolecules,1996(29):2327-3230. |
| [7] | H S,White;R M,Mather;P T Jeon;H,S Phillips,J Lichtenhan .Nanoscale reinforcement of polyhedral oligomeric silsesquioxane(POSS)in polyurethane elactnmer[J].Polymer International,2000,49(05):437-440. |
| [8] | 卢婷利 .含倍半硅氧烷有机无机杂化高分子材料的研究[D].西安:西北工业大学,2005. |
| [9] | H Y Xu;S W Kuo;J S Lee;F C Chang.Glass transition temperatures of poly(hydroxystyrene-covinylpyrrolidone-co-polyhedral oligosilsesquioxanes)[J].Polymer,2000(43):5117-5124. |
| [10] | 张亚峰,孙陆逸,刘安华,龚克成.笼型六面体倍半硅氧烷衍生物制备聚合物纳米复合材料[J].化学世界,2001(02):98-102. |
| [11] | Jiwon Choi;Jason Harcup;Albert F.Yee;Quan Zhu;Richard M.Laine .Organic/inorganic hybrid composites from cubic silsesquioxanes[J].Journal of the American Chemical Society,2001(46):11420-11430. |
| [12] | Norbert Auner;Jan W. Bats;Dimitris E. Katsoulis;Michitaka Suto;Ronald E. Tecklenburg;Gregg A. Zank .Chemistry of Hydrogen-Octasilsesquioxane: Preparation and Characterization of Octasilsesquioxane-Containing Polymers[J].Chemistry of Materials,2000(11):3402-3418. |
| [13] | H Y Xu;S W Kuo;F C Chang.Significant glass transition temperature increase based on oligomeric silsequioxane(POSS)copolymer through hydrogen polyhedral bonding[J].Polymer Bulletin,2002(48):469-474. |
| [14] | Shipp DA.;Matyjaszewski K.;Wang JL. .Synthesis of acrylate and methacrylate block copolymers using atom transfer radical polymerization[J].Macromolecules,1998(23):8005-8008. |
| [15] | Lee A.;Lichtenhan JD. .Viscoelastic responses of polyhedral oligosilsesquioxane reinforced epoxy systems[J].Macromolecules,1998(15):4970-4974. |
| [16] | P T Mather;H G Jeon;A R Uribe;T S Haddad,J D Liehtenhan.Meehanieal Relaxation and Mierostrueture of Poly(norbomyl-POSS)CoPolymers[J].Macromolecules,1999(32):1194-1203. |
| [17] | L Zheng;R J Farris;E B Coughlin.Novel Polyolefin Nanocomposites:Synthesis And Characterizations of Metalloeene-Catalyzed Polyolefin Polyhe-dral Oligomeric Silsesquioxane Copolymere[J].Macromolecules,2001(34):8034-8039. |
| [18] | 胡立江,张兴文,黄玉东,孙德智,孙毅.有机/无机杂化纳米结构单元的空间构型研究--Ⅰ.乙烯基倍半硅氧烷梯型结构的量子力学确定[J].中国科学B辑,2004(03):202-210. |
| [19] | 卢婷利,梁国正,宫兆合,任鹏刚,张增平.含倍半硅氧烷的杂化聚合物[J].高分子通报,2004(01):15-20. |
| [20] | 沈媛 .笼型倍半硅氧烷在蒙脱土中的插层自组装及聚苯乙烯复合材料的研究[D].北京化工大学,2007. |
| [21] | 邢文涛 .酸催化聚倍半硅氧烷涂层的制备及其耐腐蚀性的研究[D].复旦大学,2008. |
| [22] | AFRL POSSTM application reseacrh.POSS Nanoteehnology Conefernce.Huntington Beach,CA[S].,2002. |
| [23] | Gonzalez R;Svejda S;Phillips S.Surface studies of space survivable hybrid organic/inorganic polymers[J].American Chemical Society Meeting Chiegao IL 26 Aug,2001 |
| [24] | R M Laine;K Y Blhoowika;T R Robinson;M L Hoppe,P Nardi,J Kajnrpe,J Uhm .Synthesis of Pentacoordineat Silieon Complexes from SiO2[J].Nature,1991,353(6345):642-644. |
| [25] | A Tsuehid;C Bolln;F G Semetz;H Frey,R Miilhaupt .Ethene and Porpene Copolymers Containing Silsesquioxnae Side Corpus[J].Macmmolecules,1997,30(10):2818-2824. |
| [26] | Kim KM.;Adachi K.;Chujo Y. .Polymer hybrids of functionalized silsesquioxanes and organic polymers utilizing the sol-gel reaction of tetramethoxysilane[J].Polymer: The International Journal for the Science and Technology of Polymers,2002(4):1171-1175. |
| [27] | Eric Devarx;Maryline Rochery;Serge Bourbigot.Polyurethane/clay and Polyurethane/POSS nanocomposites as flame retarded coating for Polyeaster and cotton fables[J].Fire and Materials,2002(26):149-154. |
| [28] | 符连社;张洪杰;邵华 等.溶胶-凝胶法制备无机/有机杂化材料研究进展[J].材料科学与工程,1999,17(01):84-88. |
| [29] | 黄娆,刘之景.新型低介电常数材料研究进展[J].微纳电子技术,2003(09):11-14,18. |
| [30] | 王献彪 .POSS基低介电多孔材料的制备表征[D].合肥:安徽大学,2004. |
| [31] | Tong Ren;Xiaoming Zhang;Jishuan Suo .Synthesis of periodic mesoporous organosilicas via the "S~+X~-I+" route[J].Microporous and Mesoporous Materials,2002(1/2):139-144. |
| [32] | M O gawa .Formation of Novel Oriented Transparent Films of Layered Silica Surfactant[J].Journal of the American Chemical Society,1994,116(17):7941-7942. |
| [33] | Jianye Wen;Garth L. Wilkes .Organic/Inorganic Hybrid Network Materials by the Sol-Gel Approach[J].Chemistry of Materials,1996(8):1667-1681. |
| [34] | 刘丰祎,符连社,王俊,张洪杰.桥联聚倍半硅氧烷的近期研究进展--单体合成及应用[J].化学通报,2003(06):382-387,403. |
| [35] | Makoto Yoshida;Paras N. Prasad .Sol-Gel-Processed SiO_2/TiO_2/Poly(vinylpyrrolidone) Composite Materials for Optical Waveguides[J].Chemistry of Materials,1996(1):235-241. |
| [36] | J V Crivello;M Rnajit .Synthesis and Photolntiiated cationicl Poylmerization of monomers with the silsesquioxnaecoer[J].Journal of Polymer Seienee Part A:Polymer Chemist,1997,35(03):407-425. |
| [37] | M Yoshid;P N Pasrda.Sol-Gel-processed SiO2/TiO2/poly(viny1 Pyrrolidone)Composite Materials for Optical waveguides[J].Chemistry of Materials,1996(08):235-241. |
| [38] | H Y Xu;S W Kuo;J S Lee;F C Chnag.Glass transition temperatures of Poly(droxyysterne-co-vinylpyrrolidone-co-polyhedral oligosilsesquioxnaes)[J].Polymer,2000(43):5117-5124. |
| [39] | Cory J. Stephanson;G. Patrick Flanagan .Synthesis of a novel anionic hydride organosiloxane presenting biochemical properties[J].International journal of hydrogen energy,2003(11):1243-1250. |
| [40] | Harris M;Chaudhary T;Drzal L et al.Silicon oxycarbide coatings on graphite fibers:chemistry,processing,and oxidation resistance[J].Materials Science and Engineering A,1995,195(01):223-226. |
| [41] | 吴蕾 .双光子吸收功能材料的合成及性能研究[D].安徽大学,2007. |
| [42] | Junxiang Zhang;Yiping Cui;Mingliang Wang;Juzheng Liu .Synthesis of double-conjugated-segment molecules and their application as ultra-broad two-photon-absorption optical limiters[J].Chemical communications,2002(21):2526-2527. |
| [43] | Zhan Y Q;Xiong Z H;Shi H Z;Zhang S T,Xu Z,Zhong G Y,He J,Zhao J M,Wang Z J,Obbard E,Ding H J,Wang X J,Ding X M .Sodium Stearate,an Effective a Mphiphilic Molecule Buffer Material Between Organic and Metal Layers in Organic Light-emitting Devices[J].Applied Physics Letters,2003,83(08):1656-1658. |
| [44] | C X Zhang;F Baboanneua;C Bonhonune;R M Laine.Highly Porous Polyhedarl Silsesquioxane Polymers.Synthesis and Characeterization[J].Journal of the American Chemical Society,1998(120):8380-8391. |
| [45] | Mather Patrick T.;Romo-Uribe A.;Haddad Timothy S.;Lichtenhan Joseph D.;Jeon Hong G. .Mechanical relaxation and microstructure of poly(norbornyl-POSS) copolymers[J].Macromolecules,1999(4):1194-1203. |
| [46] | Wei-Jung Lin;Wen-Chang Chen;Wen-Chung Wu;Yu-Hua Niu;Alex K.-Y.Jen .Synthesis and Optoelectronic Properties of Starlike Polyfluorenes with a Silsesquioxane Core[J].Macromolecules,2004(7):2335-2341. |
| [47] | Hunter J Murfee;Travis P S Thoms;John Greaves.New Metallodendrimers Containing an Octakis(diphenylphosphino Functionalized Silsesquioxane Core and Ruthenium(Ⅱ)-Based Chromophores[J].Inorganic Chemistry,2000(39):5209-5217. |
| [48] | Feng Gao;Bill M. Culbertson;Yuhua Tong;Scott R. Schricker .Evaluation of multi-methacrylates copolymerized with methacryl-poss for potential organic-inorganic hybrid dental restorative materials[J].Polymer Preprints,2000(1):580-581. |
| [49] | Jonghee Lee;Hoon-Je Cho;Byung-Jun Jung .Stabilized Blue Luminescent Polyfluorenes:Introducing Polyhedral Oligomeric Silsesquioxane[J].Macromolecules,2004(23):8523-8529. |
| [50] | Mantz R A;Jones P F;Chaffee K P.Thermolysis of polyhedral oligomerie Silsesquioxane(P055)Macromers and POSS-Siloxane Copolymers[J].Chemistry of Materials,1996(08):1250. |
| [51] | Xu HY.;Kuo SW.;Lee JS.;Chang FC. .Preparations, thermal properties, and T-g increase mechanism of inorganic/organic hybrid polymers based on polyhedral oligomeric silsesquioxanes[J].Macromolecules,2002(23):8788-8793. |
| [52] | Rob W.J.M.Hanssen;Rutger A.van Santen;Hendrikus C.L.Abbenhuis .The Dynamic Status Quo of Polyhedral Silsesquioxane Coordination Chemistry[J].European journal of inorganic chemistry,2004(4):675-683. |
| [53] | Jeon H G;Mather P T;Haddad T S.Polymer International[J].,2000(49):453. |
| [54] | Chyi-Ming Leu;G Mahesh Reddy;Kung-Hwa Wei;Ching-Fong Shu.Synthesis and dielectrics of polyimide-chain-end tethered polyhedral oligomeric silsesquioxane nanocomposite[J].Chemistry of Materials,2003(15):2261-2265. |
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