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以乙烯为碳源、多壁碳纳米管为载体负载钴作为催化剂,利用CVD法制备出了高质量的多壁碳纳米管.利用扫描电子显微镜(SEM)对催化剂的形貌进行了表征,利用透射电子显微镜(TEM)、X射线衍射仪(XRD)以及差热-热重(TG-DTA)方法对产物进行了表征.发现在最佳裂解温度770℃下制备的多壁碳纳米管直径分布均匀、曲率小、纯净、产率高,更重要的是不具有难处理的氧化物(如Al2O3)载体,充分体现了碳纳米管作为载体的优越性.

参考文献

[1] Iijima S .Helical microtubules of graphitic carbon[J].Nature,1991,354:56.
[2] Thess A;Lee R;Nikolaev P et al.Crystalline ropes of metallic carbon nanotubes[J].Science,1996,273:483.
[3] Shi Z J;Lian Y F;Zhou X H et al.Mass-production of single-wall carbon nanotubes by arc discharge method[J].Carbon,1999,37(09):1449.
[4] A carbon-nanotube-based nanorelay[J].Applied physics letters,2003(8):1287-1289.
[5] Qian D;Dickey E C .[J].Journal of Microscopy,2001,204(01):39.
[6] Liu C;Fan Y Y;Liu M et al.Hydrogen storage in single-walled carbon nanotubes atroomtemperature[J].Science,1999,286:1127.
[7] Xu D S;Guo G L;Gui L L et al.[J].Applied Physics Letters,1999,75:481.
[8] Pan Z W;Xie S S;Chang B H et al.Direct growth of aligned open carbon nanotubes by chemical vapor deposition[J].Chemical Physics Letters,1999,299:97.
[9] 丁佩,张红瑞,郭新勇,杜祖亮,梁二军.催化剂对碳纳米管产率及质量的影响[J].光散射学报,2003(01):42-47.
[10] Li W Z;Xie S S;Qian L X et al.L arge-Scale Synthesis of Aligned Carbon Nanotubes[J].Science,1996,274:1701.
[11] Cassel A M;Raymakers J A;Kong J et al.[J].Journal of Physical Chemistry B,1999,103:6484.
[12] Chen P.;Lin J.;Li H.;Tan KL.;Wu X. .Comparative studies on the structure and electronic properties of carbon nanotubes prepared by the catalytic pyrolysis of CH4 and disproportionation of CO[J].Carbon: An International Journal Sponsored by the American Carbon Society,2000(1):139-143.
[13] 李志飞,罗国华,魏飞,向兰,邓祥义.催化剂对纳米聚团床法制备的纳米碳材料形貌的影响[J].催化学报,2002(02):173-178.
[14] Lim S;Shimizu A;Yoon S H et al.High yield preparation of tubular carbon nanofibers over supported Co-Mo catalysts[J].CARBON,2004,42:1273.
[15] Reshetenko T V;Avdeeva L B;Ismagilov Z R et al.Catalytic filamentous carbon as supports for nickel catalysts[J].CARBON,2004,42:143.
[16] Otsuka K;Abe Y;Kanai N et al.Synthesis of carbon nanotubes on Ni/carbon-fiber catalysts under mild conditions[J].CARBON,2004,42:727.
[17] Planeix J M;Coustel N;Coq B et al.Application of carbon nanotubes as supports in heterogeneous catalysis[J].Journal of the American Chemical Society,1994,116:7935.
[18] Luo JZ.;Leung YL.;Au CT.;Gao LZ. .The decomposition of NO on CNTs and 1 wt% Rh/CNTs[J].Catalysis Letters,2000(1/2):91-97.
[19] Yun CAI,Jing Dong LIN,Hong Bo CHEN,Hong Bin ZHANG,Guo Dong LIN,Dai Wei LIAO.Novel Ru - K/Carbon Nanotubes Catalyst for Ammonia Synthesis[J].中国化学快报(英文版),2000(04):373-374.
[20] Zhan Y;Zhang H B;Lin G D et al.[J].Applied Catalysis A:General,1999,187:213.
[21] 李春华,姚可夫,阮殿波,梁吉,吴德海.以镍/碳纳米管催化剂制备碳纳米管[J].中国科学E辑,2002(06):735-739.
[22] Kong J;Soh H T;Cassell A M et al.Synthesis of individual singlewalled carbon nanotubes on patterned silicon wafers[J].Nature,1998,395:878.
[23] 吕德义,徐丽萍,徐铸德,葛忠华.CVD法制备碳纳米管的TG-DTA研究--温度对CVD法制备碳纳米管的影响[J].化学物理学报,2002(02):118-122.
[24] 邹红玲,杨延莲,武斌,卿泉,李清文,张锦,刘忠范.CVD法制备单壁碳纳米管的纯化与表征[J].物理化学学报,2002(05):409-413.
[25] 陈萍,张鸿斌,林国栋,蔡启瑞.催化裂解CH4或CO制碳纳米管结构性能的谱学表征[J].高等学校化学学报,1998(05):765-769.
[26] Baker R T K .[J].Carbon,1989,27:315.
[27] Lee C J;Park J .[J].Applied Physics Letters,2000,77(21):3397.
[28] Zhang L N;Zhou J P et al.[J].Journal of Chromatography A,1998,816:131.
[29] Tang C C;Ding X X;Gan Z W et al.[J].Carbon,2002,40:2497.
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