2013年12月在呼和浩特市主城区9个环境空气监测点位同步采集PM10样品,对PM10浓度和16种多环芳烃的浓度、污染特征进行了分析,使用特征比值和主成分分析对多环芳烃来源进行了解析.9个监测点位的PM10浓度介于23.5-322 μg·m-3之间,16种多环芳烃总量介于5.34-850 ng·m-3之间.荧蒽、芘、苯并[a]蒽、(屈)、苯并[b]荧蒽、苯并[a]芘、苯并[g,h,i]苝和茚并[1,2,3-ed]芘等多环芳烃单体浓度较高,这8种多环芳烃占多环芳烃总浓度的80.4％.主成分分析所获得污染源结果和特征比值法定性判断出的污染源结果一致,燃烧源、机动车尾气源和石油源为主要污染源,分别贡献61.3％、16.0％和10.4％.
参考文献
| [1] | Fei Chen;Wei Hu;Qin Zhong.Emissions of particle-phase polycyclic aromatic hydrocarbons (PAHs) in the Fu Gui-shan Tunnel of Nanjing, China[J].Atmospheric research,2013Apr.(Apr.):53-60. |
| [2] | M.S. Callen;J.M. Lopez;A. Iturmendi;A.M. Mastral.Nature and sources of particle associated polycyclic aromatic hydrocarbons (PAH) in the atmospheric environment of an urban area[J].Environmental Pollution,2013Dec.(Dec.):166-174. |
| [3] | X.L.ZHANG;S.TAG;W.X.LIU;Y.YANG;Q.ZUO.Source Diagnostics of Polycyclic Aromatic Hydrocarbons Based on Species Ratios:A Multimedia Approach[J].Environmental Science & Technology: ES&T,200523(23):9109-9114. |
| [4] | E.G. Sanderson;A. Raqbi;A. Vyskocil;J.-P. Farant.Comparison of particulate polycyclic aromatic hydrocarbon profiles in different regions of Canada[J].Atmospheric environment,200421(21):3417-3429. |
| [5] | Ilias G. Kavouras;Petros Koutrakis;Manolis Tsapakis;Evaggelia Lagoudaki;Euripides G. Stephanou;Dietrich Von Baer;Pedro Oyola.Source apportionment of urban particulate aliphatic and polynuclear aromatic hydrocarbons (PAHs) using multivariate methods[J].Environmental Science & Technology: ES&T,200111(11):2288-2294. |
| [6] | Athanasios Katsoyiannis;Andrew J. Sweetman;Kevin C.Jones.PAH Molecular Diagnostic Ratios Applied to Atmospheric Sources: A Critical Evaluation Using Two Decades of Source inventory and Air Concentration Data from the UK[J].Environmental Science & Technology: ES&T,201120(20):8897-8906. |
| [7] | 周海军;孙文静;团良;石艳菊;何江.重点污染源企业周边农田土壤中多环芳烃污染水平与风险评价[J].环境化学,2013(10):1976-1982. |
| [8] | 王超;张霖琳;刀谞;吕怡兵;滕恩江;李国刚.京津冀地区城市空气颗粒物中多环芳烃的污染特征及来源[J].中国环境科学,2015(1):1-6. |
| [9] | 郭红连;陆晨刚;余琦;陈立民.上海大气可吸入颗粒物中多环芳烃（PAHs）的污染特征研究[J].复旦学报（自然科学版）,2004(6):1107-1112. |
| [10] | 陈敏;张卫东;周志恩;郭志顺.重庆市春季不同功能区PM10中多环芳烃的污染特征[J].中国环境监测,2013(1):43-48. |
| [11] | 钱冉冉;闫景明;吴水平;王新红.厦门市冬春季灰霾期间大气PM10中多环芳烃的污染特征及来源分析[J].环境科学,2012(9):2939-2945. |
| [12] | 李伟芳;彭跃;赵丽娟;仇伟光;白志鹏.东北地区城市大气颗粒物中多环芳烃的污染特征[J].中国环境监测,2013(1):13-17. |
| [13] | Yunker MB.;Macdonald RW.;Vingarzan R.;Mitchell RH.;Goyette D. Sylvestre S..PAHs in the Fraser River basin: a critical appraisal of PAH ratios as indicators of PAH source and composition [Review][J].Organic Geochemistry: A Publication of the International Association of Geochemistry and Cosmochemistry,20024(4):489-515. |
| [14] | Li GC;Xia XH;Yang ZF;Wang R;Voulvoulis N.Distribution and sources of polycyclic aromatic hydrocarbons in the middle and lower reaches of the Yellow River, China[J].Environmental Pollution,20063(3):985-993. |
| [15] | LI Xing-hong;MA Ling-ling;LIU Xiu-fen;FU Shan;CHENG Hang-xin;XU Xiao-bai.Polycyclic aromatic hydrocarbon in urban soil from Beijing, China[J].环境科学学报(英文版),2006(05):944-950. |
| [16] | 秦传高;钟秦;胡伟;石莹莹;张强华.南京市可吸入颗粒物中多环芳烃的源解析[J].环境化学,2008(3):318-321. |
| [17] | 丁潇;白志鹏;韩斌;张杰峰.鞍山市大气PM10中多环芳烃（PAHs）的污染特征及其来源[J].环境科学研究,2011(2):162-171. |
| [18] | 段永红;陶澍;王学军;李本纲;徐福留;刘文新;曹军;朱利中;骆永明.天津表土中多环芳烃含量的空间分布特征与来源[J].土壤学报,2005(6):942-947. |
| [19] | Mohamad Pauzi Zakaria;Hideshige Takada;Shinobu Tsutsumi;Kei Ohno;Junya Yamada;Eriko Kouno;Hidetoshi Kumata.Distribution of polycyclic aromatic hydrocarbons (PAHs) in rivers and estuaries in Malaysia: a widespread input of petrogenic PAHs[J].Environmental Science & Technology: ES&T,20029(9):1907-1918. |
| [20] | Simcik MF;Lioy PJ;Eisenreich SJ*.Source apportionment and source/sink relationships of PAHs in the coastal atmosphere of Chicago and Lake Michigan[J].Atmospheric environment,199930(30):5071-5079. |
| [21] | ROY M. HARRISON;D. J. T. SMITH;L. LUHANA.Source Apportionment of Atmospheric Polycyclic Aromatic Hydrocarbons Collected from an Urban Location in Birmingham, U.K.[J].Environmental Science & Technology: ES&T,19963(3):825-832. |
| [22] | H. Guo;S C. Lee;K.F. Ho;X.M. Wang;S.C. Zou.Particle-associated polycyclic aromatic hydrocarbons in urban air of Hong Kong[J].Atmospheric environment,200338(38):5307-5317. |
| [23] | 张巍;张树才;万超;岳大攀;叶友斌;胡俊栋;王开颜;高艳;王学军.北京城市道路地表径流及相关介质中多环芳烃的源解析[J].环境科学,2008(6):1478-1483. |
| [24] | Ruchaya Boonyatumanond;Gullaya Wattayakorn;Ayako Togo;Hideshige Takada.Distribution and origins of polycyclic aromatic hydrocarbons (PAHs) in riverine, estuarine, and marine sediments in Thailand[J].Marine pollution bulletin,20068(8):942-956. |
上一张
下一张
上一张
下一张
计量
- 下载量()
- 访问量()
文章评分
- 您的评分：
-
10%
-
20%
-
30%
-
40%
-
50%